It depends on your criteria. Aluminum is lighter and steel is stronger and harder. The whole Alzheimer's thing is controversial but stainless steel is widely considered safe. I personally prefer stainless steel because of its durability and I feel more comfortable boiling water in it if I have to.

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Stainless steel is the better material. Food grade stainless steel, like those of Klean Kanteen water bottles, are light, strong, BPA free, and unlike aluminum, are highly corrosion resistant.

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I have experience with both, and while aluminum is lighter steel definitely holds up better. My aluminum bottles, Siggs included, will dent if dropped on a hard surface. Stainless on the other hand is much stronger. I also tend to lean towards Klean Kanteens because they fit in a cup/bottle holder better in the car and on a backpack.

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Aluminum bottles like "Sigg:"http://mysigg.com/index.asp?PageAction=COMPANY bottles have a food grade inner coating that prevents leaching and is taste and scent neutral.

Aluminum bottles are lighter, but dent more easily.

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